Experimental Investigation of Synthetic Graphene Oxide-Hexamethyldisilazane Nanofluid Injection to Improve Oil Recovery

Document Type : Research Article

Authors

1 Department of Chemical Engineering, Kermanshah Branch, Islamic Azad University, Kermanshah, I.R. IRAN

2 Department of Petroleum Engineering, Research Institute of petroleum Industry, Tehran, I.R. IRAN

3 Department of Chemistry, Kermanshah Branch, Islamic Azad University, Kermanshah, I.R. IRAN

Abstract

One of the effective methods in the process of enhanced recovery of oil reservoirs is applying the nanotechnology to alter the wettability of the reservoir rock. In this study, the wettability alteration was investigated using synthetic graphene oxide-Hexamethyldisilazane (GO-HMDS). For this purpose, XRD and FTIR analyzes were used to identify the synthesized structure. In the present study, the effect of concentration (0.05, 0.1 and 0.2 wt% GO-HMDS) were investigated using the zeta potential analysis, Interfacial Tension (IFT), and contact angle. Subsequently, the concentration of 0.2% was determined as a powerful sample in altering the wettability of the reservoir rock through the zeta potential analysis. This sample was used for tests of contact angle and interfacial tension. In addition the zeta potential of the sample was measured by -36 mv. Moreover, the contact angle between the reservoir rock and the graphene oxide- (Hexamethyldisilazane) solution for 0.2 wt.% GO-HMDS solution decreased from 161 to 44 degrees. On the other hand, it is in agreement the results of the zeta potential and Interfacial Tension (IFT) examines. Therefore, the synthesized nanofluid reduces the and Interfacial Tension (IFT), contact angle, and wettability alteration toward the water-wet of the carbonate core.

Keywords

Main Subjects


[1] Dahle G.S., Investigation of how Hydrophilic Silica Nanoparticles Affect Oil Recovery in Berea Sandstone, Master thesis, Petroleum Engineering and Applied Geophysics, Trondheim, (2014).
[2] Ju B., Shugao D., Zhian L., Tiangoa Z., Xiatao S., Xiaofeng Q., A Study of Wettability and Permeability Change Caused by Adsorption of Nanometer Structured Polysilicon on the Surface of Porous Media, SPE Journal., Melbourne, Australia, 8–10 October, (2002).
[3] Rezaei-Namin A., Rashidi  A., Gharesheikhlou A.A., Ghasemy  E., Jalilian  M., Experimental Application of Functionalized N-Doped Graphene for Improving Enhanced Oil Recovery, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 581: 123-801 (2019).
[4] Radnia H., Rashidi A., Nazar A.R.S., Eskandari M.M., Jalilian M., A Novel Nanofluid based on Sulfonated Graphene for Enhanced Oil Recovery, Journal of Molecular Liquids, 271: 795-806 (2018).
[5] Kamal M.S., Sultan A.S., Al-Mubaiyedh U.A., Hussein I.A., Review on Polymer Flooding: Rheology, Adsorption, Stability, and Field Applications of Various Polymer Systems, Polymer Reviews, 55(3): 491–530 (2015).
[6] Gong H., Li Y., Dong M., Ma S., Liu W., Effect of Wettability Alteration on Enhanced Heavy Oil Recovery by Alkaline Flooding, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 488: 28–35 (2016).
[7] Bayat M., Lashkarbolooki M., Hezave A.Z., Ayatollahi S., Investigation of Gas Injection Flooding Performance as Enhanced Oil Recovery Method, Journal of Natural Gas Science and Engineering, 29: 37–45 (2016).
[8] Lu T., Li Z., Li S., Wang P., Wang Z., Liu S., Enhanced Heavy Oil Recovery after Solution Gas Drive by Water Flooding, Journal of Petroleum Science and Engineering, 137: 113–124 (2016).
[9] Liyanage P.J., Lu J., Arachchilage G.W.P., Weerasooriya U.P., Pope G.A., A Novel Class of Large-Hydrophobe Tristyrylphenol (TSP) Alkoxy Sulfate Surfactants for Chemical Enhanced Oil Recovery, Journal of Petroleum Science and Engineering, 128: 73–85 (2015).
[10] Goudarzi A., Delshad M., Mohanty K. K., Sepehrnoori K., Surfactant Oil Recovery in Fractured Carbonates: Experiments and Modeling of Different Matrix Dimensions, Journal of Petroleum Science and Engineering, 125: 136–145 (2015).
[11] Wang C., Li X., Li  P., Niu Y., Interactions between Fluorinated Cationic Guar Gum and Surfactants in the Dilute and semi-Dilute Solutions, Carbohydrate Polymers, 99: 638– 645 (2014).
[12]  Rostami A., Zargar G., Takassi M.A., Moradi S., Jabari B., Evaluation of a New Agent for Wettability Alteration during Enhanced Oil Recovery, Iran. J. Chem. Chem. Eng., 39(5): 333-341 (2020).
[14] Kamari A., Gharagheizi F., Shokrollahi A., Arabloo M., Mohammadi A.H., Integrating a Robust Model for Predicting Surfactant-Polymer Flooding Performance, Journal of Petroleum Science and Engineering, 137: 87–96 (2016).
[15] Bikkina P., Wan J., Kim Y., Kneafsey T.J., Tokunaga T.K., Influence of Wettability and Permeability Heterogeneity on Miscible CO2 Flooding Efficiency, Fuel, 166: 219–226 (2015).
[16] Ahmadi M.A., Shadizadeh S.R., Implementation of a Highperformance Surfactant for Enhanced Oil Recovery from Carbonate Reservoirs, Journal of Petroleum Science and Engineering, 110: 66–73 (2013).
[17] Ahmadi M.A., Shadizadeh S.R., Experimental Investigation of Adsorption of a New Nonionic Surfactant on Carbonate Minerals, Fuel, 104: 462–467 (2013).
[18] Zendehboudi S., Ahmadi M.A., Rajabzadeh A.R., Mahinpey N., Chatzis I., Experimental Study on Adsorption of a New Surfactant onto Carbonate Reservoir Samples-Application to EOR, Canadian Journal of Chemical Engineering, 91(8): 1439–1449 (2013).
[19] Kamal M.S., Sultan A.S., Al-Mubaiyedh U.A., Hussein I.A., Y Feng., Rheological Properties of Thermoviscosifying Polymers in High-temperature and High-salinity Environments, Canadian Journal of Chemical Engineering, 93(7): 1194–1200 (2015).
[20] Kamal M.S., Sultan A.S., Al-Mubaiyedh U.A., Hussien I.A., Pabon M., Evaluation of Rheological and Thermal Properties of a New Fluorocarbon Surfactant-Polymer System for EOR Applications in High-Temperature and High-Salinity Oil Reservoirs, Journal of Surfactants and Detergents, 17(5): 985–993 (2014).
[21] Wang Y., Feng Y., Wang B., Lu Z., A Novel Thermoviscosifying Water-Soluble Polymer: Synthesis and Aqueous Solution Properties, Journal of Applied Polymer Science, 116(6): 3516–3524 (2010).
[22] Wu Y., Shuler P.J., Blanco M., Tang Y., Goddard-III W.A., An Experimental Study of Wetting Behavior and Surfactant EOR in Carbonates with Model Compounds, SPE Journal, 13(1): 26–34 (2008).
[23] Lan Q., Yang F., Zhang S., Liu S., Xu J., Sun D., Synergistic Effect of Silica Nanoparticle and Cetyltrimethyl Ammonium Bromide on the Stabilization of O/W Emulsions, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 302(1-3): 126–135 (2007).
[24] Hashemi R., Nassar N.N., Almao P.P., Nanoparticle Technology for Heavy Oil In-Situ Upgrading and Recovery Enhancement: Opportunities and Challenges, Applied Energy, 133: 374–387 (2014).
[25] Bhuiyan M.H.U., Saidur R., Amalina M.A., Mostafizur R.M., Islam A., Effect of Nanoparticles Concentration and their Sizes on Surface Tension of Nanofluids, Procedia Engineering, 105: 431–437 (2015).
[26] Taylor R., Coulombe S., Otanicar T., Phelan P., Gunawan A., Lv W., Rosengarten G., Prasher R., Tyagi H., Small Particles, Big Impacts: A Review of the Diverse Applications of Nanofluids, Journal of Applied Physics, 113(1): 011301 (2013).
[28] Zargartalebi M., Barati N., Kharrat R., Influences Ofhydrophilic and Hydrophobic Silica Nanoparticles on Anionic Surfactant Properties: Interfacial and Adsorption Behaviors, Journal of Petroleum Science and Engineering, 119: 36– 43 (2014).
[29] Morrow N., Wettability and Its Effect on Oil Recovery, Journal of Petroleum Technology., 42(12): 1476–1484 (1990).
[30] Ali J.A., Kolo K.,  Khaksar-Manshad A., Stephen K.D., Potential Application of Low-Salinity Polymeric-Nanofluid in Carbonate Oil Reservoirs: IFT Reduction, Wettability Alteration, Rheology and Emulsification Characteristics, Journal of Molecular Liquids, 284: 735-747 (2019).
[32] علائی م.، افضلی تبار م.، رشیدی ع.، تعیین نانوساختار کربنی برتر برای سنتز سیلیکا نانوهیبرید برای ازدیاد برداشت از مخازن نفت، نشریه شیمی و مهندسی شیمی ایران، (4)40: 215 تا 223 (1398).
[33] Jalali A., Firozjaii A.M., Shadizadeh S.R., Experimental Investigation on New Derived Natural Surfactant: Wettability Alteration, IFT Reduction, and Core Flooding in Oil Wet Carbonate Reservoir, Energy Sources, Part A: Recovery, Utilization, and Environmental Effects, 45(2): 4282-4292 (2019).
[34] Ali J.A., Kolo  K.,  Khaksar-Manshad A., Stephen K.D., Potential Application of Low-Salinity Polymeric-Nanofluid in Carbonate Oil Reservoirs: IFT Reduction, Wettability Alteration, Rheology and Emulsification Characteristics, Journal of Molecular Liquids, 284: 735-747 (2019).
[35] Ogolo N.A., Olafuyi O.A., Onyekonwu M.O., Enhanced Oil Recovery using Nanoparticles, SPE Journal, Al-Khobar, Saudi Arabia, 8–11 April, (2012).
[36] Al-Anssari S., Barifcani A., Wang S., Maxim L., Iglauer S., Wettability Alteration of Oil-Wet Carbonate by Silica Nanofluid, Journal of Colloid and Interface Science, 461: 435–442 (2016).
[37] Roustaei A., Moghadasi J., Bagherzadeh H., Shahrabadi A., An Experimental Investigation of Polysilicon Nanoparticles' Recovery Efficiencies through Changes in Interfacial Tension and Wettability Alteration, SPE Journal, Noordwijk, Netherlands, 12–14 June, (2012).
[38] Yoo M.J., Park H.B., Effect of Hydrogen Peroxide on Properties of Graphene Oxide in Hummers Method, Carbon, 141: 515-522 (2019).
[39] Zaaba N.I., Foo K.L.,  Hashim  U., Tan S.J., Liu W.W., Voon C.H., Synthesis of Graphene Oxide using Modified Hummers Method: Solvent Influence, Procedia Engineering, 184: 469-477 (2017).
[40] Peng C., Xiong Y., Liu Z., Zhang F., Ou E., Qian J., Xiong Y., Xu W., Bulk Functionalization of Graphene using Diazonium Compounds and Amide Reaction, App. Sur. Sci., 280: 914-919 (2013).
[41] Tuteja S.K., Kukkar M., Suri C., Paul A., Deep A., One Step in-Situ Synthesis of Amine Functionalized Graphene for Immunosensing of Cardiac Marker cTnI, Biosens Bioelectron, 66: 129–135 (2015).
[42] Mondragon R., Julia J.E., Barba A., Jarque J.C., Characterization of Silica–Water Nanofluids Dispersed with an Ultrasound Probe: A Study of their Physical Properties and Stability, Powder Technol., 224: 138–146 (2012).
[43] Chai H., Lin Y., Evans D. G., Li D., Synthesis and UV Absorption Properties of 2- Naphthylamine-1,5-Disulfonic Acid Intercalated Zn-Al Layered Double Hydroxides, Ind. Eng. Chem. Res., 47: 2855–2860 (2008).
[44] Refat M.S., Adam A.M.A., Sharshar T., Saad H.A., Eldaroti H.H., Utility of Positron Annihilation Lifetime Technique for the Assessment of Spectroscopic Data of Some Charge-Transfer Complexes Derived from N-(1-Naphthyl)Ethylenediamine Dihydrochloride, Spectrochim. Acta Mol. Biomol. Spectrosc., 122: 34-47 (2014).
[45] Radnia H., Solaimany-Nazar A.R., Rashidi A.M., Experimental Assessment of Graphene Oxide Adsorption onto Sandstone Reservoir Rocks through Response Surface Methodology, Journal of the Taiwan Institute of Chemical Engineers, 8080: 34-45 (2017).